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Feingold, G., 2003: Modeling of the first indirect effect: Analysis of measurement requirements. Geophys. Res. Lett., 30, No. 19, 1997, doi:10.1029/2003GL017967.

   

[1] We investigate the extent to which aerosol extinction is a suitable proxy for the aerosol affecting drop formation. First we use multiple realizations of a cloud model to investigate the sensitivity of cloud drop effective radius re to aerosol parameters (size distribution and composition) and dynamical parameters (updraft and liquid water content). In general, re is most sensitive to cloud liquid water, a parameter often ignored in indirect effect analyses. The relative importance of the other parameters varies for different conditions but aerosol concentration Na is consistently important. Updraft plays an increasingly important role under high aerosol loadings. A breakdown of the individual aerosol terms contributing to drop size change shows that use of aerosol extinction as a proxy for size distribution and composition tends to underestimate the magnitude of the first indirect effect. This may influence interpretation of current satellite and surface remote measurements of the indirect effect. INDEX TERMS: 0305 Atmospheric Composition and Structure: Aerosols and particles (0345, 4801); 0320 Atmospheric Composition and Structure: Cloud physics and chemistry; 1610 Global Change: Atmosphere (0315, 0325); 1640 Global Change: Remote sensing. Citation: Feingold, G., Modeling of the first indirect effect: Analysis of measurement requirements, Geophys. Res. Lett., 30(19), 1997, doi:10.1029/2003GL017967, 2003. [3] In situ measurements, both surface-based and airborne, address the fundamental microphysical processes by measuring size distribution and composition. However, for climate monitoring purposes it is not feasible to perform global measurements of these parameters with the detail applied to in situ measurements. Satellites use passive remote sensors to measure aerosol optical depth ta which is used as an indicator of aerosol effects on cloud drop size. Satellites provide global coverage of aerosols and clouds but do not measure details of aerosol size and composition. In addition, aerosol measurements are pathintegrated and not collocated with clouds. Surface based remote sensors [e.g., Feingold et al., 2003] measure aerosol extinction a beneath clouds, cloud droplet size, and liquid water path (LWP) in a single column of air at scales pertinent to cloud drop formation (100 m). Again, a (local ta) is used as a proxy for size distribution and composition. [4] The question explored in this paper is whether proxies such as a are adequate, or alternatively, what set of measurements needs to be made to provide useful assessments of the first indirect effect. One can view this as an endeavour to guide measurement strategies in the coming years.

   

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